학술논문

Observations of atmospheric chemical deposition to high Arctic snow
Document Type
Report
Author abstract
Source
Atmospheric Chemistry and Physics. May 10, 2017, Vol. 17 Issue 9, 5775
Subject
Snow -- Environmental aspects
Atmospheric circulation -- Observations
Earth sciences
Observations
Environmental aspects
Language
English
ISSN
1680-7316
Abstract
Rapidly rising temperatures and loss of snow and ice cover have demonstrated the unique vulnerability of the high Arctic to climate change. There are major uncertainties in modelling the chemical depositional and scavenging processes of Arctic snow. To that end, fresh snow samples collected on average every 4 days at Alert, Nunavut, from September 2014 to June 2015 were analyzed for black carbon, major ions, and metals, and their concentrations and fluxes were reported. Comparison with simultaneous measurements of atmospheric aerosol mass loadings yields effective deposition velocities that encompass all processes by which the atmospheric species are transferred to the snow. It is inferred from these values that dry deposition is the dominant removal mechanism for several compounds over the winter while wet deposition increased in importance in the fall and spring, possibly due to enhanced scavenging by mixed-phase clouds. Black carbon aerosol was the least efficiently deposited species to the snow.
Byline: Katrina M. Macdonald, Sangeeta Sharma, Desiree Toom, Alina Chivulescu, Sarah Hanna, Allan K. Bertram, Andrew Platt, Mike Elsasser, Lin Huang, David Tarasick, Nathan Chellman, Joseph R. McConnell, Heiko Bozem, [...]