학술논문

Enhancing Scattering Circular Dichroism of Chiral Substrate via Mie Resonances
Document Type
Periodical
Author
Source
IEEE Photonics Journal IEEE Photonics J. Photonics Journal, IEEE. 16(1):1-6 Feb, 2024
Subject
Engineered Materials, Dielectrics and Plasmas
Photonics and Electrooptics
Manganese
Scattering
Substrates
Optical scattering
Optical polarization
Nanoparticles
Nonlinear optics
Mie scattering
chirality
circular dichroism
T-matrix
high-index particle
Language
ISSN
1943-0655
1943-0647
Abstract
Chirality plays a pivotal role in the interaction between light and matter, yet detecting chiral signals from natural materials remains a challenge, necessitating the enhancement of their intensity. In this study, we present an approach to investigate substrate chirality through exploiting light scattering from Mie particles. To comprehensively analyze the scattering phenomenon, we theoretically derive the T-matrix for a nonchiral Mie sphere positioned on a chiral substrate. Unlike the Mie sphere in free space, our derivation accounts for the intricate coupling between the scattered light by the sphere and the reflected light by the substrate. Employing the T-matrix framework, we calculate the scattering power and circular dichroism spectra. Our findings reveal a remarkable augmentation of chiral signals originating from the substrate, thanks to the Mie resonance within high-index spheres. This research underscores the feasibility of probing local chiral properties in the vicinity of a sample surface, promising new insights into chiral interactions at the nanoscale.