부산대학교 도서관

The discovery of superconductivity in the infinite-layer (IL) nickelates provides a new platform and angle of view to study the long-standing problem of high temperature superconductivity . Many models were proposed to understand its superconducting mechanisms based on the calculated electronic structure, and the multiple Fermi surfaces and multiple orbitals involved create complications and controversial conclusions. Over the past 5 years, the lack of direct measurements of the electronic structure has hindered the understanding of nickelate superconductors. Here, we fill this gap by preparing IL LaNiO$_2$ and La$_{0.8}$Ca$_{0.2}$NiO$_2$ thin films with superior surface quality and measuring their electronic structure by angle-resolved photoemission spectroscopy (ARPES).The Fermi surface consists of a large three-dimensional hole pocket primarily contributed by Ni-3$d_{x^2-y^2}$ states, and a small electron pocket at the Brillouin zone (BZ) corner. The hole pocket exhibits a two-dimensional character over approximately 80% of the Brillouin zone, and its Fermi surface topology and band dispersion closely resemble those observed in hole-doped cuprates, suggesting their superconducting mechanisms may be alike. Yet this hole pocket shows strong three-dimensional character near $k_z=\pi$, which deviates from previous calculations and adds new facets to the superconductivity in IL nickelates. The experimental electronic structure represents a pivotal step toward a microscopic understanding of the IL nickelate family and its superconductivity.
Comment: 19 pages, 5 figures