학술논문

Vertically Processed GaInP/InP Tandem-Junction Nanowire Solar Cells
Document Type
Source
ACS Applied Nano Materials NanoLund: Centre for Nanoscience. 7(2):2352-2358
Subject
GaInP
InP
nanowire solar cell
photovoltaics
tandem junction
Naturvetenskap
Fysik
Den kondenserade materiens fysik
Natural Sciences
Physical Sciences
Condensed Matter Physics
Language
English
ISSN
2574-0970
Abstract
We present vertically processed photovoltaic devices based on GaInP/InP tandem-junction III-V nanowires (NWs), contacting approximately 3 million NWs in parallel for each device. The GaInP and InP subcells as well as the connecting Esaki tunnel diode are all realized within the same NW. By processing GaInP/InP tandem-junction NW solar cells with varying compositions of the top junction GaInP material, we investigate the impact of the GaInP composition on the device performance. External quantum efficiency (EQE) measurements on devices with varying GaInP composition provide insights into the performance of the respective subcells, revealing that the GaInP subcell is current-limiting for all devices. I-V measurements under AM1.5G illumination confirm voltage addition of the subcells, resulting in an open-circuit voltage of up to 1.91 V. However, the short-circuit current density is low, ranging between 0.24 and 3.44 mA/cm2, which leads to a resulting solar conversion efficiency of up to 3.60%. Our work shows a path forward toward high-efficiency NW photovoltaics and identifies critical issues that need improvement.