학술논문

Fabrication of Nitrogen-Doped Graphene Quantum Dots-Cu2O Catalysts for Enhanced Photocatalytic Hydrogen Evolution
Document Type
Article
Source
NANO, 13(8), pp.108-114 Aug, 2018
Subject
자연과학
Language
English
ISSN
1793-2920
Abstract
Development of efficient visible light driven photocatalysts for water splitting has attracted great research interest. Herein, a novel H2-producing nitrogen-doped graphene quantum dots (NGQDs)-Cu2O was successfully constructed and synthesized. The as-prepared NGQDs-Cu2O photocatalysts were benefited for light harvesting and charge separation and showed highly efficient photocatalytic property for hydrogen production by water splitting. Results displayed that the amount of NGQDs exhibited significant influence for H2 production, and the optimum sample of 3%NGQDs-Cu2O performed the highest hydrogen-evolution rate of 22.6 μmol h -1 g -1, which was about 2 times higher than that of the pure Cu2O (10.1 μmol h -1 g -1). By further study, the enhanced photocatalytic performance could be ascribed to the crucial role of NGQDs, which widely improve the separation of photogenerated electron-hole pair's.