학술논문

Concentration Variations of Total Organic Nitrates at Fukue Island, Nagasaki, Japan: Relationships between Transport Time and Atmospheric Lifetime / 長崎県福江島における有機硝酸の濃度変動―輸送時間と大気寿命の関係―
Document Type
Journal Article
Source
大気環境学会誌 / Journal of Japan Society for Atmospheric Environment / Taiki Kankyo Gakkaishi. 2023, 59(1):1
Subject
concentration variation
lifetime
long-range transport
total organic nitrates
total peroxy nitrates
transport time
Language
Japanese
ISSN
1341-4178
2185-4335
Abstract
Continuous observations of organic nitrates were conducted from February to May 2022 at Fukue Island, Nagasaki, Japan. The average concentrations of PNs (Total peroxy nitrates) and ONs (Total organic nitrates) during the observation period were 0.44±0.33 and 0.26±0.14 ppbv (1σ), respectively. The air mass origins arriving at Fukue were classified into the following seven groups: Russia, Northern China (NC), Korea, Northern China/Korea (NC+KR), Southern China, Japan, and Ocean, using backward trajectory analyses, and the concentration variations for each air mass origin were investigated. In February and March, PNs and ONs concentrations from NC were the highest of the seven air mass origins. In April and May, however, PNs and ONs concentrations from NC decreased, while those from NC+KR were the highest. Such concentration variations would be attributed to the relationship between the atmospheric lifetime and the transport time from the Asian continent to Fukue. In April and May, the air masses from NC have long transport times and most of PNs would be lost before arriving at Fukue Island, while the air masses from NC+KR have shorter transport times than those from NC, and the percentage of PNs loss during the transport would be low.