학술논문

THz-pump / MIR-probe nanospectroscopy on Si-doped GaAs-InGaAs core-shell nanowires
Document Type
Conference
Source
2023 48th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) Infrared, Millimeter, and Terahertz Waves (IRMMW-THz), 2023 48th International Conference on. :1-2 Sep, 2023
Subject
Aerospace
Bioengineering
Communication, Networking and Broadcast Technologies
Components, Circuits, Devices and Systems
Engineered Materials, Dielectrics and Plasmas
Fields, Waves and Electromagnetics
Photonics and Electrooptics
Signal Processing and Analysis
Heat pumps
Free electron lasers
Optical pumping
Plasmas
Nanowires
Effective mass
Electric fields
Language
ISSN
2162-2035
Abstract
We report on first THz-pump / MIR-probe SNOM studies on Si-doped GaAs-InGaAs core-shell NWs utilizing THz radiation from the free-electron laser FELBE. Upon intraband THz-pump we observe a red shift of the NW plasma resonance in both amplitude and phase spectra, while a controlled interband optical pumping induces a blue shift of the resonance. In both cases, the signal exponentially decays with a time constant of 4-5 ps. We attribute the blue shift to the contribution of photogenerated charge carriers, while the red shift is assigned to the heating of electrons in the conduction band accelerated by the THz electric field of the pump pulses and the subsequent increase of their effective mass due to the nonparabolic $\Gamma$-valley dispersion.