학술논문

Coherent Light Emitters From Solution Chemistry: Inorganic II–VI Nanocrystals and Organometallic Perovskites
Document Type
Periodical
Source
IEEE Journal of Selected Topics in Quantum Electronics IEEE J. Select. Topics Quantum Electron. Selected Topics in Quantum Electronics, IEEE Journal of. 23(5):1-14 Jan, 2017
Subject
Engineered Materials, Dielectrics and Plasmas
Photonics and Electrooptics
Optical films
Optical pumping
Excitons
Stimulated emission
Absorption
Vertical cavity surface emitting lasers
Colloidal quantum dots
distributed feedback
exciton
nanocrystals
nanoplatelets
optical gain
perovskite
photonic crystal
vertical-cavity surface-emitting laser
Language
ISSN
1077-260X
1558-4542
Abstract
Semiconductor lasers are the prime example of compact coherent light-emitters having developed into mature technologies with ubiquitous presence in applications across much of the optical spectrum. Yet there are reasons to explore new materials, both to access those parts of the spectrum not fully accessible by these inorganic single crystal devices, while exploring alternative high throughput methods of material synthesis. In this paper, we focus on solution-processed thin film nanocrystal materials as possible candidates to expand the material repertoire of semiconductor lasers. We review work on inorganic II–VI compound colloidal quantum dots and nanoplatelets and then present recent work in our laboratory on organometallic perovskites, which have gained significant attention quite recently by their promise as high performance photovoltaic solar cells. We concentrate on fundamentals of the optical gain and means of integrating the solution grown nano/microcrystalline thin films into high-Q cavities to identify prime challenges ahead to turn these intriguing materials into viable laser devices.