학술논문

Monolithic Carbon Nanotube Film Thermoelectric Generator
Document Type
Periodical
Source
IEEE Transactions on Electron Devices IEEE Trans. Electron Devices Electron Devices, IEEE Transactions on. 71(2):1179-1184 Feb, 2024
Subject
Components, Circuits, Devices and Systems
Engineered Materials, Dielectrics and Plasmas
Substrates
Temperature measurement
Fabrication
Electrodes
Carbon nanotubes
Optical filters
Resistance
Monolithic
sacrificial molding technique
single-walled carbon nanotube (SWCNT)
thermoelectric generator (TEG)
thermoelements
Language
ISSN
0018-9383
1557-9646
Abstract
The design and development of a thermoelectric generator (TEG) with minimal internal resistance is crucial for achieving high output power in self-powered wearable technologies. This work presents a novel flexible TEG comprising single-walled carbon nanotube (SWCNT) thermoelements, fabricated through a sacrificial molding process. Different from the traditional TEG structural design, our TEG’s ${p}$ - and ${n}$ -type SWCNT thermoelements are formed monolithically without any interconnections. This integration eliminates the presence of internal resistance within the device. Equipped with eight pairs of the ${p}$ - and ${n}$ -type SWCNT thermoelements, the TEG exhibits an open-circuit voltage ( ${V}_{\text {oc}}{)}$ of ~21.82 mV and an internal resistance of $\sim 16.56~\Omega $ , corresponding to a maximum output power of approximately $7.19~\mu \text{W}$ at a temperature gradient $(\Delta {T})$ of 50 °C. Additionally, the TEG demonstrated its capability to harvest energy from a fingertip, generating a ${V}_{\text {oc}}$ of around 2.58 mV at a $\Delta {T}$ of 8.8 °C. These results highlight the potential of the monolithically formed SWCNT thermoelements for achieving high-power density TEGs.