학술논문

Characterization of morphology-dependent transport in lead-halide perovskite printed films using time-resolved terahertz spectroscopy
Document Type
Conference
Source
2023 48th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) Infrared, Millimeter, and Terahertz Waves (IRMMW-THz), 2023 48th International Conference on. :1-2 Sep, 2023
Subject
Aerospace
Bioengineering
Communication, Networking and Broadcast Technologies
Components, Circuits, Devices and Systems
Engineered Materials, Dielectrics and Plasmas
Fields, Waves and Electromagnetics
Photonics and Electrooptics
Signal Processing and Analysis
Printing
Location awareness
Spectroscopy
Morphology
Optical variables measurement
Position measurement
Lead
Language
ISSN
2162-2035
Abstract
We report on position-dependent measurements of photocarrier transport using time-resolved terahertz spectroscopy (TRTS) across a slot-die printed perovskite film of varying morphology. Using the Drude-Smith model for the photoconductivity spectra we report maximum intrinsic mobilities of $540 \pm 20$ ${\mathrm {cm}}^{2} {\mathrm {V}}^{-1} {\mathrm {s}}^{-1}$. In addition, we measure variation across the film in the extracted mobilities and the localization c-parameter, correlated with complementary measurements of the film morphology and optical properties. To the best of our knowledge this is the first TRTS study performed on perovskite films produced using a slot-die printing technique.