학술논문

Influence of water uptake on the aerosol particle light scattering coefficients of the Central European aerosol
Document Type
article
Source
Tellus: Series B, Chemical and Physical Meteorology, Vol 66, Iss 0, Pp 1-14 (2014)
Subject
aerosol particle light scattering
hygroscopic growth
scattering enhancement
aerosol mass spectrometer
field measurements
optical closure study
Meteorology. Climatology
QC851-999
Language
English
ISSN
1600-0889
Abstract
The influence of aerosol water uptake on the aerosol particle light scattering was examined at the regional continental research site Melpitz, Germany. The scattering enhancement factor f(RH), defined as the aerosol particle scattering coefficient at a certain relative humidity (RH) divided by its dry value, was measured using a humidified nephelometer. The chemical composition and other microphysical properties were measured in parallel. f(RH) showed a strong variation, e.g. with values between 1.2 and 3.6 at RH=85% and λ=550 nm. The chemical composition was found to be the main factor determining the magnitude of f(RH), since the magnitude of f(RH) clearly correlated with the inorganic mass fraction measured by an aerosol mass spectrometer (AMS). Hysteresis within the recorded humidograms was observed and explained by long-range transported sea salt. A closure study using Mie theory showed the consistency of the measured parameters.