학술논문

Quantitative Long-Term Monitoring of the Circulating Gases in the KATRIN Experiment Using Raman Spectroscopy
Document Type
article
Author
Max AkerKonrad AltenmüllerArmen BeglarianJan BehrensAnatoly BerlevUwe BessererBenedikt BieringerKlaus BlaumFabian BlockBeate BornscheinLutz BornscheinMatthias BöttcherTim BrunstThomas C. CaldwellSuren ChilingaryanWonqook ChoiDeseada D. Díaz BarreroKarol DebowskiMarco DeffertMartin DescherPeter J. DoeOtokar DragounGuido DrexlinStephan DybaFrank EdzardsKlaus EitelEnrico EllingerRalph EngelSanshiro EnomotoMariia FedkevychArne FeldenJoseph F. FormaggioFlorian FränkleGregg B. FranklinFabian FriedelAlexander FulstKevin GaudaWoosik GilFerenc GlückRobin GrößleRainer GumbsheimerVolker HannenNorman HaußmannKlaus HelbingStephanie HickfordRoman HillerDavid HillesheimerDominic HinzThomas HöhnThibaut HoudyAnton HuberAlexander JansenChristian KarlJonas KellererLuke KippenbrockManuel KleinChristoph KöhlerLeonard KöllenbergerAndreas KopmannMarc KorzeczekAlojz KovalíkBennet KraschHolger KrauseLuisa La CascioThierry LasserreThanh-Long LeOndřej LebedaBjoern LehnertAlexey LokhovMoritz MachatschekEmma MalcherekAlexander MarstellerEric L. MartinMatthias MeierChristin MelzerSusanne MertensKlaus MüllerSimon NiemesPatrick OelpmannAlexander OsipowiczDiana S. ParnoAlan W.P. PoonJose M. Lopez PoyatoFlorian PriesterOliver RestMarco RölligCarsten RötteleR.G. Hamish RobertsonCaroline RodenbeckMilos RyšavỳRudolf SackAlejandro SaenzPeter SchäferAnna Schaller (née Pollithy)Lutz SchimpfKlaus SchlösserMagnus SchlösserLisa SchlüterMichael SchrankBruno SchulzMichal SefčíkHendrik Seitz-MoskaliukValérian SibilleDaniel SiegmannMartin SlezákFelix SpanierMarkus SteidlMichael SturmMenglei SunHelmut H. TelleLarisa A. ThorneThomas ThümmlerNikita TitovIgor TkachevDrahoš VénosKathrin ValeriusAna P. Vizcaya HernándezMarc WeberChristian WeinheimerChristiane WeissStefan WelteJürgen WendelJohn F. WilkersonJoachim WolfSascha WüstlingWeiran XuYung-Ruey YenSergey ZadoroghnyGenrich Zeller
Source
Sensors, Vol 20, Iss 17, p 4827 (2020)
Subject
Raman spectroscopy
tritium
gas composition monitoring
KATRIN
Chemical technology
TP1-1185
Language
English
ISSN
1424-8220
Abstract
The Karlsruhe Tritium Neutrino (KATRIN) experiment aims at measuring the effective electron neutrino mass with a sensitivity of 0.2 eV/c2, i.e., improving on previous measurements by an order of magnitude. Neutrino mass data taking with KATRIN commenced in early 2019, and after only a few weeks of data recording, analysis of these data showed the success of KATRIN, improving on the known neutrino mass limit by a factor of about two. This success very much could be ascribed to the fact that most of the system components met, or even surpassed, the required specifications during long-term operation. Here, we report on the performance of the laser Raman (LARA) monitoring system which provides continuous high-precision information on the gas composition injected into the experiment’s windowless gaseous tritium source (WGTS), specifically on its isotopic purity of tritium—one of the key parameters required in the derivation of the electron neutrino mass. The concentrations cx for all six hydrogen isotopologues were monitored simultaneously, with a measurement precision for individual components of the order 10−3 or better throughout the complete KATRIN data taking campaigns to date. From these, the tritium purity, εT, is derived with precision of −3 and trueness of −3, being within and surpassing the actual requirements for KATRIN, respectively.