학술논문

Cavity-mediated thermal control of metal-to-insulator transition in 1T-TaS2
Document Type
Article
Source
Nature; October 2023, Vol. 622 Issue: 7983 p487-492, 6p
Subject
Language
ISSN
00280836; 14764687
Abstract
Placing quantum materials into optical cavities provides a unique platform for controlling quantum cooperative properties of matter, by both weak and strong light–matter coupling1,2. Here we report experimental evidence of reversible cavity control of a metal-to-insulator phase transition in a correlated solid-state material. We embed the charge density wave material 1T-TaS2into cryogenic tunable terahertz cavities3and show that a switch between conductive and insulating behaviours, associated with a large change in the sample temperature, is obtained by mechanically tuning the distance between the cavity mirrors and their alignment. The large thermal modification observed is indicative of a Purcell-like scenario in which the spectral profile of the cavity modifies the energy exchange between the material and the external electromagnetic field. Our findings provide opportunities for controlling the thermodynamics and macroscopic transport properties of quantum materials by engineering their electromagnetic environment.