학술논문

Nonperturbative dynamic photon absorption of quantum wells.
Document Type
Article
Source
Journal of Applied Physics. 5/15/2006, Vol. 99 Issue 10, p103104. 7p. 6 Graphs.
Subject
*QUANTUM wells
*QUANTUM theory
*FREE electron lasers
*ELECTRONS
*PHYSICAL & theoretical chemistry
Language
ISSN
0021-8979
Abstract
Optical photoresponse of quantum wells in the nonperturbative regime has been studied by high-power and ultrafast-oscillating free-electron laser (FEL) experiments, which revealed a profound deviation of the nonlinear power from conventional perturbative multiple photon absorption processes. By combining the experimental and theoretical works we have shown that the nonperturbative solution of the time-dependent Schrödinger equation is essential to understand the experimental observations. Optical transitions of electrons are dynamic. One photon is absorbed or emitted when an electron transits from one electron state to the other. The rates of absorption and emission are proportional to the time interval in the femtosecond time scale. In the picosecond time scale, multiphoton processes emerge. The strong and fast-oscillating FEL source intensifies the dynamic photon absorption and emission processes in the quantum wells, resulting in a much enhanced nonlinearity in the photoresponse spectrum. [ABSTRACT FROM AUTHOR]