학술논문

Large third-order optical nonlinearity in (Pb,La)(Zr,Ti)O3 ferroelectric thin film.
Document Type
Article
Source
Journal of Applied Physics. 12/15/2006, Vol. 100 Issue 12, p126101. 3p. 4 Graphs.
Subject
*FERROELECTRIC thin films
*THIN films
*OPTICAL properties
*NONLINEAR optics
*PEROVSKITE
*SPUTTERING (Physics)
*OPTICAL constants
*REFRACTIVE index
Language
ISSN
0021-8979
Abstract
Ferroelectric (Pb0.92La0.08)(Zr0.65Ti0.35)O3 (PLZT) film with good surface morphology and perovskite structure was grown in situ on quartz substrate by radio-frequency magnetron sputtering at 650 °C. The fundamental optical constants (the band gap energy, linear refractive index, and absorption coefficient) of the film are obtained by optical transmittance measurement. The third-order nonlinear optical properties of the films were investigated by the Z-scan technique. The magnitude and sign of the nonlinear refractive index n2 were determined, as was the negative sign, which indicated a self-defocusing optical nonlinearity. A large nonlinear refractive index as high as 1.21×10-6 esu is displayed in the film. All results show that PLZT ferroelectric thin film has potential applications in nonlinear optical devices. [ABSTRACT FROM AUTHOR]