학술논문

Suppressed Superconductivity in Ultrathin Mo2N Films due to Pair-Breaking at the Interface.
Document Type
Article
Source
Journal of Superconductivity & Novel Magnetism. Jul2022, Vol. 35 Issue 7, p1775-1780. 6p.
Subject
*THIN films
*SUPERCONDUCTIVITY
*SUPERCONDUCTING transition temperature
*TUNNELING spectroscopy
*SCANNING tunneling microscopy
*DENSITY of states
*SURFACE topography
Language
ISSN
1557-1939
Abstract
A strong disorder characterized by a small product of the Fermi vector kF and the electron mean free l drives superconductors towards insulating state. Such disorder can be introduced by making the films very thin. Here, we present 3-nm Mo2N film with kF*l ~ 2 with a resistive superconducting transition temperature Tc = 2 K heavily suppressed in comparison with the bulk Tc. Superconducting density of states (DOS) with smeared gap-like peaks and in-gap states, so called Dynes DOS, is observed by the low-temperature tunneling spectroscopy despite a sharp resistive transition. By scanning tunneling microscope, the spectral maps are obtained and related to the surface topography. The maps show a spatial variation of the superconducting energy gap on the order of 20% which is not accidental but well correlates with the surface corrugation: protrusions reveal larger gap, smaller spectral smearing, and smaller in-gap states. In agreement with our previous measurements on ultrathin MoC films, we suggest that the film-substrate interface introducing the local pair-breaking is responsible for the observed effects and generally for the suppression of the superconductivity in these ultrathin films. [ABSTRACT FROM AUTHOR]