학술논문

Altering Terahertz Sound Propagation in a Liquid upon Nanoparticle Immersion.
Document Type
Article
Source
Nanomaterials (2079-4991). Jul2022, Vol. 12 Issue 14, pN.PAG-N.PAG. 12p.
Subject
*ACOUSTIC wave propagation
*INELASTIC scattering
*X-ray scattering
*TERAHERTZ materials
*SOUND waves
*PHYSICISTS
Language
ISSN
2079-4991
Abstract
One of the grand challenges of new generation Condensed Matter physicists is the development of novel devices enabling the control of sound propagation at terahertz frequency. Indeed, phonon excitations in this frequency window are the leading conveyor of heat transfer in insulators. Their manipulation is thus critical to implementing heat management based on the structural design. To explore the possibility of controlling the damping of sound waves, we used high spectral contrast Inelastic X-ray Scattering (IXS) to comparatively study terahertz acoustic damping in a dilute suspension of 50 nm nanospheres in glycerol and on pure glycerol. Bayesian inference-based modeling of measured spectra indicates that, at sufficiently large distances, the spectral contribution of collective modes in the glycerol suspension becomes barely detectable due to the enhanced damping, the weakening, and the slight softening of the dominant acoustic mode. [ABSTRACT FROM AUTHOR]