학술논문

Development of high-performance membrane-electrode assembly in unitized regenerative fuel cells
Document Type
Article
Source
Journal of Industrial and Engineering Chemistry, 80(0), pp.527-534 Dec, 2019
Subject
화학공학
Language
English
ISSN
1876-794X
1226-086X
Abstract
In this work, we investigated the membrane-electrode assembly (MEA) parameters of an oxygenelectrode to develop a high-performance unitized regenerative fuel cell (URFC) that can be operated infuel cell (FC) and water electrolysis (WE) mode. The MEA parameters including gas diffusion layer,ionomer content, oxygen reduction reaction (ORR) type, oxygen evolution reaction (OER) catalyst, andcatalyst loading were optimized by calculating the round-trip efficiency of URFC. The performance in FCmode was largely affected by the MEA parameters compared to that of the WE mode performance. The FCmode performance is crucial for the achievement of high URFC performance. The optimized round-tripefficiency was 49% at 500 mA cm 2, which is comparable or superior to that reported in literature. Thisresult can be attributed to the highly efficient MEA structure suitable for bifunctional catalysts toparticipate in both ORR and OER.