학술논문

Accurate γ-ray spectrometry measurements of the half-life of 92Sr
Document Type
Article
Source
Applied Radiation & Isotopes. Oct2008, Vol. 66 Issue 10, p1450-1458. 9p.
Subject
*HALF-life (Nuclear physics)
*GAMMA ray spectrometry
*RADIOISOTOPE decay
*NUCLEAR fuels
*STRONTIUM
*BETA decay
*NUCLEAR counters
Language
ISSN
0969-8043
Abstract
Abstract: Studies of the nuclear fuel cycle require an accurate knowledge of the energy release from the decay of radioactive nuclides produced in a reactor, including precise half-life data for the short-lived radionuclides. Moreover, short-lived fission products are crucial for fission rate distribution measurements performed in low-power facilities, such as EOLE and MINERVE of CEA Cadarache [Fougeras, P., 2005. EOLE, MINERVE and MASURCA facilities and their associated neutron experimental programs. In: 13th International Conference on Nuclear Engineering, Beijing, China, 16–20 May 2005], and their nuclear decay data need to be known to high precision. For these reasons, the half-life of 92Sr has been measured to solve a recently observed inconsistency identified with the quoted value in the main nuclear applications libraries (including JEFF3.1): T 1/2=2.71±0.01h [Parsa, B., Ashari, A., Goolvard, L., Nobar, Y.M., 1971. Decay scheme of 2.71h 92Sr. Nucl. Phys. A 175, 629–640]. An overestimation of 4.5% has been identified in this work, based on two independent methods. Specific γ-ray spectrometry measurements on activated fissile foils have been carried out, using two HPGe detectors. Influencing factors such as net area measurements of photopeaks, pulse pile-up accuracy and dead time corrections in the presence of decaying activity are discussed. A new value has been obtained by combining eight series of measurements: T 1/2=2.594±0.006h. The uncertainty has been reduced by a factor of two with respect to previous evaluations. This measured value also shows good agreement with the most recent studies of T 1/2=2.627±0.009h [Nir-El, Y., 2003. Private Communications. Soreq Research Centre, Yavne, Israel]. [Copyright &y& Elsevier]